Radiological Assessment

Radioactivity release is one of the safety aspects for several DBA scenarios and some DEC scenarios: The following cases may be examples of DBA events with radiological consequences:

  • LOCAs with radionuclides escaping into the containment and releases into the environment through design containment leakages
  • Accidents with leaks from the primary circuit bypassing the containment, such as instrument line rupture and PRISE leaks. Primary to secondary leaks (PRISE) remain one of the most serious events which can threaten the defence in depth of nuclear power plants and jeopardize safety.
  • Leaks from the primary circuit during maintenance, refuelling or other outages.

This group of accidents, more or less leads to radioactivity releases from the fuel and the reactor coolant, their transport through the primary circuit, their release and transport to the containment and to the radiological source term released into the environment. The relevant acceptance criterion is:

“The release of radioactive material shall not result in offsite doses in excess of specific limits.”

Calculated doses must be below the limits for DBAs, assuming an event generated iodine spike and an equilibrium iodine concentration for continued power operation, and considering actual operational limits and conditions for the primary and secondary coolant activity. The radiological consequences for the environment depend primarily on short-term releases of iodine and longer-term releases of caesium. In practical terms, iodine releases determine short-term management of the accident while caesium releases determine medium- and long-term management of the accident.

In addition to engineering and procedures which reduce the risk and severity of accidents, all plants have guidelines for severe accident management or mitigation (SAM). Severe accident scenarios commonly used evolved from those developed in the Reactor Safety Study, which is often refered to as WASH-1400. The following cases may be examples of DEC events:

  • LB-LOCA with loss of all ac power (AB accident)
  • Containment bypass accidents (mode V)

Acceptance criteria for severe accidents are less prescriptive than the criteria for DBAs. Typically, the criterion is considered in relation to the very low probability associated with an severa accident.

Examples of more specific criteria are as follows:

  • There should be no failure of the containment because of pressure and temperature loads.
  • There should be no immediate health effects on the population.
  • For long term effects the 137Cs release limit needs to be below the prescribed value

Source Term

In nuclear safety, the source term refers to the magnitude and mix of the radionuclides released from the fuel and reactor coolant, which would be available for escape to the environment from a nuclear reactor that has undergone a severe accident.

Source term is a very important part of reactor safety analysis. The reactor accidents that could in principle have the largest source term for a given LWR plant are those in which severe fuel damage occurs in addition to one of three classes of containment impairment.

The accidents are those that:

  • might threaten containment integrity early in the history of the event;
  • might remobilize large amounts of fission products in late containment failure;
  • might lead to bypass of the containment function.

Radioactive material escaping from the containment is often referred to as the “radiological release to the environment.” The radiological release is obtained from the containment leak rate and a knowledge of the airborne radioactive inventory in the containment atmosphere. The radioactive inventory within containment is referred to as the “in-containment accident source term.”

For all accidents with the potential for release of radioactivity into the environment, the class of accidents that had the shortest time until the first fuel rod failed was the design basis LOCA. As might be expected, the time until cladding failure is very sensitive to the design of the reactor, the type of accident assumed, and the fuel rod design. In particular, the maximum linear heat generation rate, the internal fuel rod pressure, and the stored energy in the fuel rod are significant considerations.

The most important ways to maintain risk and the source term at low levels are design features and accident management methods that would prevent severe core damage. The next most important are design features and accident management methods that would preserve the integrity and the functions of the containment.

For analysis of the source term, specific groupings of postulated initiating events may be appropriate to adequately address different pathways that could lead to the release of radioactive material to the environment. Special attention should be paid to accidents in which the release of radioactive material could bypass the containment, because of the potentially severe consequences even in the case of relatively small releases.

Radionuclides of greatest concern in reactor safety

The radionuclides in a nuclear reactor that could most affect public health if released are the fission products and the actinides produced by neutron transmutation. It must be noted, irradiated nuclear fuel contains a large number of different isotopes that contribute to radiological hazards. Fission fragments with a short half-life are much more radioactive (at the time of production) and contribute significantly to local hazards, but will obviously lose its share rapidly. On the other hand, fission fragments and transuranic elements with a long half-life are less radioactive (at the time of production) and produce acute hazards, but will obviously lose its share more slowly. In considering the hazards of these radionuclides release in an accident sequence, a number of factors determine their importance. These are especially:

  • Core inventory. Core inventory (i.e. total activity) depends on the balance between formation and decay.
  • Chemical and physical properties. Chemical and physical properties of radionuclides determine cumulation and various reactions that may occur during accidents. This could affect transports and absorption of radionuclides after their release.
  • Biological characteristics. Radioactive isotopes that were ingested or taken in through other pathways will gradually be removed from the body via bowels, kidneys, respiration and perspiration. This means that a radioactive substance can be expelled before it has had the chance to decay.

Radionuclides of greatest concern in reactor safety are summarized in the table, these are:

  • Iodine-131. I-131 decays with a half-life of 8.02 days with beta particle and gamma emissions. As it decays, it may cause damage to the thyroid. The primary risk from exposure to high levels of I-131 is the chance occurrence of radiogenic thyroid cancer in later life. For I-131, ICRP has calculated that if you inhale 1 x 106 Bq, you will receive a thyroid dose of HT = 400 mSv (and weighted whole-body dose of 20 mSv).
  • Strontium-90. Sr-90, Ra-226 and Pu-239 are radionuclides known as bone-seeking radionuclides. These radionuclides have long biological half-lives and are serious internal hazards. Once deposited in bone, they remain there essentially unchanged in amount during the lifetime of the individual.
  • Caesium-137. Caesium-137 is among the most problematic of the short-to-medium-lifetime fission products because it easily moves and spreads in nature due to the high water solubility. The biological behaviour of caesium is similar to that of potassium.
  • Tritium. Tritium emits low-energy beta particles with a short range in body tissues and, therefore, poses a risk to health as a result of internal exposure only following ingestion in drinking water or food, or inhalation or absorption through the skin. The tritium taken into the body is uniformly distributed among all soft tissues. According to the ICRP, a biological half-time of tritium is 10 days for HTO and 40 days for OBT (organically bound tritium) formed from HTO in the body of adults. As a result, for an intake of 1 x 109 Bq of tritium (HTO), an individual will get a whole-body dose of 20 mSv.

radionuclides in reactors - reactor safety

See also: Dangerous quantities of radioactive material (D-values), EPR-D-VALUES 2006. IAEA 2006

 
References:
Nuclear and Reactor Physics:
  1. J. R. Lamarsh, Introduction to Nuclear Reactor Theory, 2nd ed., Addison-Wesley, Reading, MA (1983).
  2. J. R. Lamarsh, A. J. Baratta, Introduction to Nuclear Engineering, 3d ed., Prentice-Hall, 2001, ISBN: 0-201-82498-1.
  3. W. M. Stacey, Nuclear Reactor Physics, John Wiley & Sons, 2001, ISBN: 0- 471-39127-1.
  4. Glasstone, Sesonske. Nuclear Reactor Engineering: Reactor Systems Engineering, Springer; 4th edition, 1994, ISBN: 978-0412985317
  5. W.S.C. Williams. Nuclear and Particle Physics. Clarendon Press; 1 edition, 1991, ISBN: 978-0198520467
  6. G.R.Keepin. Physics of Nuclear Kinetics. Addison-Wesley Pub. Co; 1st edition, 1965
  7. Robert Reed Burn, Introduction to Nuclear Reactor Operation, 1988.
  8. U.S. Department of Energy, Nuclear Physics and Reactor Theory. DOE Fundamentals Handbook, Volume 1 and 2. January 1993.

Nuclear Safety:

  1. IAEA Safety Standards, Safety of Nuclear Power Plants: Design, SSR-2/1 (Rev. 1). VIENNA, 2016.
  2. IAEA Safety Standards, Safety of Nuclear Power Plants: Commissioning and Operation, SSR-2/2 (Rev. 1). VIENNA, 2016.
  3. IAEA Safety Standards, Deterministic Safety Analysis for Nuclear Power Plants, SSG-2 (Rev. 1). VIENNA, 2019.
  4. IAEA TECDOC SERIES, Considerations on the Application of the IAEA Safety Requirements for the Design of Nuclear Power Plants, IAEA-TECDOC-1791. VIENNA, 2016.
  5. Safety Reports Series, Accident Analysis for Nuclear Power Plants with Pressurized Water Reactors. ISBN 92–0–110603–3. VIENNA, 2003.
  6. Appendix A to 10 CFR Part 50, “General Design Criteria for Nuclear Plants.”
  7. NUREG-0800, Standard Review Plan for the Review of Safety Analysis Reports for Nuclear Power Plants: LWR Edition.
  8. Nuclear Power Reactor Core Melt Accidents, Science and Technology Series. IRSN – Institute for Radiological Protection and Nuclear Safety. ISBN: 978-2-7598-1835-8
  9. ANSI ANS 51.1: Nuclear Safety Criteria for the Design of Stationary Pressurized Water Reactor Plants, 1983.

See above:

Nuclear Safety